Thermosensitive hydrogels to deliver reactive species generated by cold atmospheric plasma: a case study with methylcellulose


Por: Solé-Martí X, Vilella T, Labay C, Tampieri F, Ginebra MP and Canal-Barnils C

Publicada: 12 jul 2022 Ahead of Print: 1 jun 2022
Resumen:
Hydrogels have been recently proposed as suitable materials to generate reactive oxygen and nitrogen species (RONS) upon gas-plasma treatment, and postulated as promising alternatives to conventional cancer therapies. Acting as delivery vehicles that allow a controlled release of RONS to the diseased site, plasma-treated hydrogels can overcome some of the limitations presented by plasma-treated liquids in in vivo therapies. In this work, we optimized the composition of a methylcellulose (MC) hydrogel to confer it with the ability to form a gel at physiological temperatures while remaining in the liquid phase at room temperature to allow gas-plasma treatment with suitable formation of plasma-generated RONS. MC hydrogels demonstrated the capacity for generation, prolonged storage and release of RONS. This release induced cytotoxic effects on the osteosarcoma cancer cell line MG-63, reducing its cell viability in a dose-response manner. These promising results postulate plasma-treated thermosensitive hydrogels as good candidates to provide local anticancer therapies.

Filiaciones:
Solé-Martí X:
 Biomaterials, Biomechanics and Tissue Engineering Group, Department of Materials Science and Engineering, and Research Centre for Biomedical Engineering (CREB), Universitat Politècnica de Catalunya (UPC), c/Eduard Maristany 14, 08019 Barcelona, Spain.

 Barcelona Research Center in Multiscale Science and Engineering, UPC, 08019 Barcelona, Spain

 Institut de Recerca Sant Joan de Déu, Santa Rosa 39-57, 08950 Esplugues de Llobregat, Spain

Vilella T:
 Biomaterials, Biomechanics and Tissue Engineering Group, Department of Materials Science and Engineering, and Research Centre for Biomedical Engineering (CREB), Universitat Politècnica de Catalunya (UPC), c/Eduard Maristany 14, 08019 Barcelona, Spain.

 Barcelona Research Center in Multiscale Science and Engineering, UPC, 08019 Barcelona, Spain

Labay C:
 Biomaterials, Biomechanics and Tissue Engineering Group, Department of Materials Science and Engineering, and Research Centre for Biomedical Engineering (CREB), Universitat Politècnica de Catalunya (UPC), c/Eduard Maristany 14, 08019 Barcelona, Spain.

 Barcelona Research Center in Multiscale Science and Engineering, UPC, 08019 Barcelona, Spain

 Institut de Recerca Sant Joan de Déu, Santa Rosa 39-57, 08950 Esplugues de Llobregat, Spain

Tampieri F:
 Biomaterials, Biomechanics and Tissue Engineering Group, Department of Materials Science and Engineering, and Research Centre for Biomedical Engineering (CREB), Universitat Politècnica de Catalunya (UPC), c/Eduard Maristany 14, 08019 Barcelona, Spain.

 Barcelona Research Center in Multiscale Science and Engineering, UPC, 08019 Barcelona, Spain

 Institut de Recerca Sant Joan de Déu, Santa Rosa 39-57, 08950 Esplugues de Llobregat, Spain

Ginebra MP:
 Biomaterials, Biomechanics and Tissue Engineering Group, Department of Materials Science and Engineering, and Research Centre for Biomedical Engineering (CREB), Universitat Politècnica de Catalunya (UPC), c/Eduard Maristany 14, 08019 Barcelona, Spain.

 Barcelona Research Center in Multiscale Science and Engineering, UPC, 08019 Barcelona, Spain

 Institute for Bioengineering of Catalonia (IBEC), Barcelona Institute of Science and Technology (BIST), c/Baldiri i Reixach 10-12, 08028 Barcelona, Spain

Canal-Barnils C:
 Biomaterials, Biomechanics and Tissue Engineering Group, Department of Materials Science and Engineering, and Research Centre for Biomedical Engineering (CREB), Universitat Politècnica de Catalunya (UPC), c/Eduard Maristany 14, 08019 Barcelona, Spain.

 Barcelona Research Center in Multiscale Science and Engineering, UPC, 08019 Barcelona, Spain

 Institut de Recerca Sant Joan de Déu, Santa Rosa 39-57, 08950 Esplugues de Llobregat, Spain
ISSN: 20474830





Biomaterials Science
Editorial
ROYAL SOC CHEMISTRY, THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND, Reino Unido
Tipo de documento: Article
Volumen: 10 Número: 14
Páginas: 3845-3855
WOS Id: 000808113200001
ID de PubMed: 35678531
imagen Green Published, hybrid

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